GNU Collaborative International Dictionary of English
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Found one definition
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Illume , v. t. [imp. & p. p. Illumed ; p. pr. & vb. n. Illuming.] [Cf. F. illuminer. See Illuminate.] To throw or spread light upon; to make light or bright; to illuminate; to illumine.Shak.1913 Webster
The mountain's brow,
Illumed with fluid gold.Thomson.1913 Webster